Speed,
Although its rare, they definitely can be out of balance. See if you can find a shop that has one of the old "on car" wheel balancers. If not, you can take the drums to a balancing shop and have them spin them and see if they are bad. ANyone that can balance a crankshaft should have an arbor for doing flywheels. You can use it to do drums. But ...... it might be cheaper in the long run to just buy new drums.
I did a set of drums for a guy about two years ago. He had problems with a Caddy that none of the tire stores could figure out and the drums were pretty far out of balance. He swears the car has never been that smooth, even when new.